CONSTITUTIVE MODELLING OF SILICONE ADHESIVE CONSIDERING MULLINS EFFECT

Guo Xin; Chen Suwen

doi:10.6052/0459-1879-23-035

Volume 55 Issue 6

Jun. 2023

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Chinese Journal of Theoretical and Applied Mechanics > 2023 > 55(6): 1308-1318. > DOI: 10.6052/0459-1879-23-035 CSTR: 32045.14.0459-1879-23-035

Guo Xin, Chen Suwen. Constitutive modelling of silicone adhesive considering Mullins effect. Chinese Journal of Theoretical and Applied Mechanics, 2023, 55(6): 1308-1318. DOI: 10.6052/0459-1879-23-035

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CONSTITUTIVE MODELLING OF SILICONE ADHESIVE CONSIDERING MULLINS EFFECT

Guo Xin^*,
Chen Suwen^{*, †, ,}

*.
College of Civil Engineering, Tongji University, Shanghai 200092, China
†.
State Key Laboratory for Disaster Reduction in Civil Engineering, Tongji University, Shanghai 200092, China

Received Date: February 06, 2023
Accepted Date: April 26, 2023
Available Online: April 27, 2023

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Abstract

Abstract

Silicone adhesive has been widely used in assembly glass curtain walls. To achieve a reliable bonding system, an effective description of material behavior is required. However, commonly used phenomenological hyperelastic models have not considered the microstructure properties of materials and cannot describe the mechanisms of their mechanical behaviors, while the classical entropic hyperelastic models often do not consider the non-affine deformation, entanglement effect or other features of polymer network. The above deficiencies make it difficult for the existing models to effectively simulate the mechanical behavior of silicone adhesive, especially the significant Mullins effect under cyclic loading. For these reasons, in this paper, based on the non-affine network model and microsphere model of polymer chain distribution, we modified the macro-micro deformation transformation and the evolution of chain conformation to consider spatial distribution of polymer chains in finite directions. Based on the modified model, network alteration functions are proposed for crosslinked and entangled network respectively using network alteration theory. These functions describe the evolution of polymer network under cyclic loading to model Mullins effect. Considering the microstructure properties and deformation mechanisms of silicone adhesive, the modified non-affine network model can describe the characteristics of polymer network, including non-affine deformation, entanglement effect, finite chain extensibility and spatial chain distribution. The comparisons with the experimental data and other model results demonstrate the capability of the modified model to accurately predict the mechanical behavior of silicone adhesive under various loading conditions, as well as the permanent set and modulus degradation of Mullins effect, which shows good potential in engineering applications.
- silicone adhesive,
- hyperelastic model,
- Mullins effect,
- non-affine network model,
- network alteration theory

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References

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CONSTITUTIVE MODELLING OF SILICONE ADHESIVE CONSIDERING MULLINS EFFECT

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